Staff Publications

Staff Publications

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    'Staff publications' is the digital repository of Wageningen University & Research

    'Staff publications' contains references to publications authored by Wageningen University staff from 1976 onward.

    Publications authored by the staff of the Research Institutes are available from 1995 onwards.

    Full text documents are added when available. The database is updated daily and currently holds about 240,000 items, of which 72,000 in open access.

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Record number 505431
Title Multimedia Environmental Fate and Speciation of Engineered Nanoparticles: A Probabilistic Modeling Approach
Author(s) Meesters, J.; Quik, J.T.K.; Koelmans, A.A.; Hendriks, A.J.; Meent, D. van de
Source Environmental Science: nano 3 (2016)4. - ISSN 2051-8153 - p. 715 - 727.
DOI https://doi.org/10.1039/C6EN00081A
Department(s) Aquatic Ecology and Water Quality Management
WIMEK
IMARES Onderzoeksformatie
Publication type Refereed Article in a scientific journal
Publication year 2016
Abstract The robustness of novel multimedia fate models in environmental exposure estimation of engineered nanoparticles (ENPs) remains unclear, because of uncertainties in the emission, physicochemical properties and natural variability in environmental systems. Here, we evaluate the uncertainty in predicted environmental concentrations (PECs) by using the SimpleBox4nano (SB4N) model. Monte Carlo (MC) simulations were performed on the environmental fate, concentrations and speciation of nano-CeO2, -TiO2 and -ZnO. Realistic distributions of uncertainty and variability were applied for all of SB4N's input and model parameter values. Environmental distribution over air, water, soil and sediment as well as nanomaterial speciation across natural colloid and coarse particles appeared to be similar for nano-CeO2, -TiO2 and -ZnO. ENPs in the atmosphere were effectively removed by deposition. ENPs in the water column were removed through hetero-aggregation–sedimentation with natural particles. ENPs accumulated in soil by attachment to grains. The sources of uncertainty and variability driving variation in PECs, which was identified in Spearman rank analysis, were related to production, emission, compartment volumes, and removal by dissolution or advection and appeared to be similar for the three ENPs. The variation in speciation within environmental compartments was influenced most by the physicochemical properties of the ENP and by model parameters that relate to the compartment of interest.
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